NDLI: Synthesis and catalytic properties of nanostructured Me/Mn$_{0.5}$Ce$_{0.5}$O$

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Synthesis and catalytic properties of nanostructured Me/Mn$_{0.5}$Ce$_{0.5}$O$_{2}$ in the oxidation of carbon monoxide

Content Provider	Springer Nature Link
Author	Liberman, E. Yu. Kleusov, B. S. Mikhailichenko, A. I. Kon’kova, T. V. Khoroshilov, A. V.
Copyright Year	2012
Abstract	The nanostructured solid solution Mn$_{0.5}$Ce$_{0.5}$O$_{2}$ is synthesized to develop effective noble metal free catalysts for the detoxification of technogenic contaminants. Its chemical and phase compositions and textural characteristics are studied by differential thermal analysis, X-ray diffraction analysis, laser mass spectrometry, and low-temperature nitrogen adsorption. The activity of the solid solution in the oxidation of carbon monoxide is determined by the flow method within a temperature range of 20–300°C at atmospheric pressure, a gas hourly space velocity of 1800 h$^{−1}$ for the following gas mixture composition, vol %: CO, 3.6; O$_{2}$, 8.0; N$_{2}$, balance. The activity of Mn$_{0.5}$Ce$_{0.5}$O$_{2}$ is shown to be appreciably higher than the activity of MnO$_{x}$ and CeO$_{2}$, and the temperature of 100% conversion is 92, 120, and 210°C, respectively. Using the solid solution as a support and the technique of impregnation, we synthesize the nanostructured catalysts Cu/Mn$_{0.5}$Ce$_{0.5}$O$_{2}$ and Ag/Mn$_{0.5}$Ce$_{0.5}$O$_{2}$, which manifest high activity in the oxidation of carbon monoxide: the temperature of 100% conversion is 77 and 85°C, respectively. The new catalysts could be of interest for the purification of industrial and motor vehicle wastes.
Starting Page	186
Ending Page	190
Page Count	5
File Format	PDF
ISSN	20700504
Journal	Catalysis in Industry
Volume Number	4
Issue Number	3
e-ISSN	20700555
Language	English
Publisher	SP MAIK Nauka/Interperiodica
Publisher Date	2012-09-15
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	cerium dioxide manganese oxide solid solution CO oxidation Catalysis
Content Type	Text
Resource Type	Article
Subject	Catalysis

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